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I'm not a doctor so this is me just trying to piece together info from other sources, but it sounds like overfeeding can cause a lot of issues that premature babies aren't developed enough to deal with on their own, like severe gas and bloating. Depending on how delicate the baby is, this might lead to a cascade of problems that are difficult to diagnose, treat, and recover from. With babies that underdeveloped, even something as benign as eating too much can become deadly.
But again, not a doctor, and a quick Google search turned up a bunch of complicated articles that don't really clarify. I just know that it was one of her strategies for worsening the babies' condition.
Depending on why the infant is in the neonatal unit, specific food can have extremely deleterious effects. Disorders of metabolism are rare, but not as rare as you think, and most are controlled with specific diets. So if she purposely fed the wrong food, and in large amounts, it could absolutely kill certain populations. If an otherwise 'healthy' infant, the most likely cause due to overfeeding would be vomiting, and then aspiration of the vomitus. Infants, especially neonates, are very unlikely to be able to protect their airway. Even if a patient is already on the operating table, survival rates of aspirating vomitus is only 50% or so. That's why you don't eat/drink before surgery, btw.
Thank you for the clarification, but my God, how awful. Those babies must have been in so much pain and distress before they died.